Research output: Contribution to journal › Article › peer-review
Research output: Contribution to journal › Article › peer-review
}
TY - JOUR
T1 - Raman Spectroscopy of Na3Co2SbO6
AU - Ponosov, Yu.
AU - Komleva, E.
AU - Pankrushina, E.
AU - Mikhailova, D.
AU - Streltsov, S.
PY - 2024/4/1
Y1 - 2024/4/1
N2 - Raman spectroscopy together with density functional calculations were used to study lattice dynamics in a layered honeycomb cobaltite Na3Co2SbO6, which can host a field-induced phase related with the Kitaev physics. We show that there develops an additional mode well above Neel temperature (at K) at 525 cm–1, which origin can be related to electronic excitation to one of doublets. Moreover, our theoretical calculations demonstrate that the highest frequency intensive mode related to the oxygen vibrations is very sensitive to type of the magnetic order. Thus, we propose to use the softening of this mode as a hallmark of the transition to a fully polarized regime, which is stabilized in Kitaev materials in strong magnetic fields.
AB - Raman spectroscopy together with density functional calculations were used to study lattice dynamics in a layered honeycomb cobaltite Na3Co2SbO6, which can host a field-induced phase related with the Kitaev physics. We show that there develops an additional mode well above Neel temperature (at K) at 525 cm–1, which origin can be related to electronic excitation to one of doublets. Moreover, our theoretical calculations demonstrate that the highest frequency intensive mode related to the oxygen vibrations is very sensitive to type of the magnetic order. Thus, we propose to use the softening of this mode as a hallmark of the transition to a fully polarized regime, which is stabilized in Kitaev materials in strong magnetic fields.
UR - http://www.scopus.com/inward/record.url?partnerID=8YFLogxK&scp=85188788587
UR - https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=tsmetrics&SrcApp=tsm_test&DestApp=WOS_CPL&DestLinkType=FullRecord&KeyUT=001194747300004
U2 - 10.1134/S0021364024600125
DO - 10.1134/S0021364024600125
M3 - Article
VL - 119
SP - 518
EP - 522
JO - JETP Letters
JF - JETP Letters
SN - 0021-3640
IS - 7
ER -
ID: 57300620